高級淨水程序之處理成效與應用粉狀活性碳薄膜反應程序去除 ...

近年來，國內淨水場之淨水程序有幾座由傳統提升為高級處理，其中包含增設了薄膜處理，然而對於生物可利用有機碳(AOC)及消毒副產物潛勢(DBPFP)之去除成效有待觀察， ... 資料載入處理中... 跳到主要內容 臺灣博碩士論文加值系統 ::: 網站導覽| 首頁| 關於本站| 聯絡我們| 國圖首頁| 常見問題| 操作說明 English |FB專頁 |Mobile 免費會員 登入| 註冊 功能切換導覽列 (165.22.106.144)您好！臺灣時間：2022/08/0615:34 字體大小：       ::: 詳目顯示 recordfocus 第1筆/ 共1筆  /1頁 論文基本資料 摘要 外文摘要 目次 參考文獻 紙本論文 QRCode 本論文永久網址: 複製永久網址Twitter研究生:黃建二研究生(外文):Chine-erHuang論文名稱:高級淨水程序之處理成效與應用粉狀活性碳薄膜反應程序去除飲用水中有機物之研究論文名稱(外文):StudyontheTreatmentEfficiencyofATPandApplicationofPowderedActivatedCarbonandMembraneBioreactortoRemoveOrganicCompoundsinDrinkingWater指導教授:樓基中指導教授(外文):Jie-ChungLou學位類別:博士校院名稱:國立中山大學系所名稱:環境工程研究所學門:工程學門學類:環境工程學類論文種類:學術論文論文出版年:2009畢業學年度:97語文別:中文論文頁數:196中文關鍵詞:薄膜生物反應程序、活性碳、生物可利用有機碳、消毒副產物、高級淨水流程外文關鍵詞:membranebioreactor、activatedcarbon、assimilableorganiccarbon、disinfectionbyproducts、advancedmembraneprocesses相關次數: 被引用:0點閱:447評分:下載:0書目收藏:0 近年來，國內淨水場之淨水程序有幾座由傳統提升為高級處理，其中包含增設了薄膜處理，然而對於生物可利用有機碳(AOC)及消毒副產物潛勢(DBPFP)之去除成效有待觀察，因此本研究分為兩大部分，第一部份為高級淨水流程之成效分析，第二部份為應用生物活性碳薄膜反應處理程序，整合兩種程序去除水中微量有機物質，並針對溶解性有機碳及生物可利用有機碳(AOC)進行效能探討。

消毒副產物部分根據本研究調查，A，B兩廠清水中總三鹵甲烷(THMs)皆以TCM(三氯甲烷)為主，濃度分別為13.97±4.18μg/L與21.49±10.59μg/L，低於國內飲用水水質標準80μg/L，此兩套高級淨水流程對於鹵化乙酸(HAA5)於A、B兩流程之清水濃度分別為17.67±14.50μg/L與33.03±16.24μg/L，結果顯示HAA5可符合目前國際飲用水水質標準。

A、B兩流程之清水HAA5物種皆以二氯乙酸(DCAA)與三氯乙酸(TCAA)為主，分別佔總量的67%及83%。

有機物部分，分析發現臭氧+活性碳生物濾床(BAC)有不錯的去除效果，但應用超過濾膜(UF)及逆滲透膜(RO)之高級流程對於生物可利用有碳(AOC)則去除效果較差，平均高達70μgacetate-C/L，無法降低至國際上文獻提及的50μgacetate-C/L水準。

根據本研究顯示高級淨水流程對水中消毒副產物有不錯的去除率，分析結果皆可降低至國內法規值與文獻建議值。

有機物部分，以臭氧配合活性碳生物濾床有一定的去除效率，但以薄膜處理之高級淨水流程可能因為水質之高硬度與高離子強度影響下造成電荷遮蔽或電荷屏障，以致於去除率不佳，本研究以生物活性碳配合薄膜過濾程序，可有效去除水中有機物並同時降低AOC值，符合文獻之建議值。

Toimprovewaterqualityofdrinkingwater,theTaiwanWaterSupplyCorp(TWSC)upgradedthreewatertreatmentplants(WTP),changingtraditionaltreatmentprocessesintotwoadvancedmembraneprocessesandoneadvancedozonationprocessesinrecentyears.Membranewatertreatmentunitsofthewatertreatmentplantcompriseultrafiltration(UF)andreverseosmosis(RO).Andtheadvancedozonationwatertreatmentunitscomprisepelletsoftening,post-ozonationandbiologicalactivatedcarbon(BAC)adsorption.Thisstudyinvestigatedtheformationofdisinfectionbyproducts(DBPs),dissolvedorganiccarbon(DOC)andassimilableorganiccarbon(AOC)attwoadvancedwatertreatmentplants(ATP)inKaohsiungCity,Taiwan,byimplementingasamplingprogram.Thepurposesofthisstudyinclude：(1)Theevaluationoftreatmentefficiencyofadvancedwatertreatmentplants.(2)Applicationofpowderedactivatedcarbonandmembranebioreactorinremovingorganiccompoundsindrinkingwater.TCMwasbyfarthepredominantspeciesinthefinishedwater,theaverageconcentrationofDPBsinthisstudyatbothplantswere13.97±4.18μg/Land21.49±10.59μg/LofTHMsforplantAandplantB,respectively.However,levelsforDPBscompoundarelowinbothplantsandlowerthanthecurrentnationaldrinkingwaterqualitystandards80μg/L.ButforanthertypicalDPBs(HAAscompounds),theaverageconcentrationswere17.67±14.50μg/Land33.03±16.24μg/LofHAA5forplantAandplantB,respectively.DCAAandTCAAwerethetwomajorspeciesofHAAsfoundinthetwowatersamplesunderstudy.Thesumsofthetwospeciesrepresentedinfinishedwaterwereabout67%and83%ofHAA5inAandplantB,respectively.TheresultsshowedthatHAA5concentrationofallsamplescouldmeetcurrentUSEPAstandardsfordrinkingwaterquality.Importantly,ourworkshowtheadvancedtreatmentprocesseshavegoodremovalonDPBsoftreatedwater.Inorganiccompoundsremoval,thereishighefficiencybyusingpost-ozonationcombinedwithBAC,butlowefficiencyformembraneprocessduetotheinhibitionofelectricalchargehappenedonsurfaceofmembrane.Thisinhibitioniscausedprobablybyhighhardnessandhighionstrengthinwater.WefoundbycombiningBACwithmembranefiltrationprocesswilleffectivelyremovetheorganiccompoundsandlowertheconcentrationofAOCforpassingthelimitvaluesuggestedinrelatedresearchesoftheworld. 目錄頁數摘要I目錄Ⅲ圖目錄Ⅷ表目錄XII第一章緒論11-1前言11-2研究緣起31-3研究目的及內容4第二章文獻回顧62-1飲用水水源現況62-1-1淨水流程82-1-2高級淨水處理程序102-2自然水體中有機物之分類及其性質232-2-1有機物之分類及其性質232-2-2水中有機物之來源與影響262-2-3原水中有機物質之替代參數292-3配水管網水質之生物穩定性問題30頁數2-3-1配水管網微生物後生長之影響因子及控制方法322-4生物可分解有機質之測定342-4-1生物可利用有機碳AOC(AssimilableOrganicCarbon)342-5消毒副產物432-5-1含氯消毒副產物442-5-2鹵化乙酸與鹵化乙酸生成潛勢472-5-3鹵化乙酸的來源492-5-4鹵化乙酸生成因素502-5-5鹵化乙酸之危害性質532-5-6鹵化乙酸之法規管制標準552-5-7鹵化乙酸生成潛勢562-6三鹵甲烷與三鹵甲烷生成潛勢572-6-1三鹵甲烷之分類572-6-2三鹵甲烷之來源592-6-3三鹵甲烷之危害性質592-6-4三鹵甲烷之法規管制標準602-6-5三鹵甲烷之生成潛勢612-7薄膜介紹及其應用61頁數2-7-1薄膜的分類與材質特性622-7-2薄膜的結構特性與選擇642-7-3薄膜過濾機制652-7-4薄膜處理所面臨之問題662-7-5薄膜於淨水廠的應用682-8薄膜生物反應器起源702-8-1MBR之種類722-8-2MBR之優點732-8-3薄膜生物反應器與粉末型活性碳78第三章研究方法803-1高級與傳統淨水場處理效能比較803-2高級淨水單元之成效評估833-3水質項目與分析方法833-4鹵化乙酸(Haloaceticacids,HAAs)843-4-1HAAs分析藥品853-4-2分析儀器及設備863-4-3採樣與保存87頁數3-4-4HAAs分析步驟883-4-5氣相層析儀分析條件913-4-6檢量線之建立913-5三鹵甲烷(Trihalomethane,THMS)923-5-1THMs分析藥品923-5-2分析儀器及設備923-5-3採樣與保存933-5-4THMs分析步驟943-5-5氣相層析儀分析條件963-5-6檢量線之建立963-6消毒副產物生成潛勢973-6-1鹵化乙酸生成潛勢973-6-2三鹵甲烷生成潛勢973-7非揮發性溶解性有機碳983-8AOC分析993-8-1純菌菌液的預先培養1013-8-2菌種活化與培養1033-8-3菌種純種鑑定與特性分析105頁數3-8-4AOC器皿之清洗方式1083-8-5AOC使用菌種其生長曲線與產率之求得1093-8-6水樣AOC之檢測方式1113-9生物活性碳薄膜實驗設備1133-9-1微生物馴養1133-9-2分析儀器與設備114第四章結果與討論1164-1菌種特性鑑定及產率(Yield)計算1164-1-1P17及NOX菌種鑑定特性1164-1-2P17及NOX之生長曲線及產率(Yield)值1174-2高級淨水場水質分析1234-2-1濁度1244-2-2總溶解固體物1254-2-3硬度1254-3消毒副產物及其潛勢1264-3-1總三鹵甲烷生成潛勢1264-3-2鹵化乙酸生成潛勢129頁數4-3-3總三鹵甲烷1334-3-4鹵化乙酸1354-4有機物1384-4-1溶解性有機碳1384-4-2生物可利用有機碳1414-5生物薄膜反應程序1454-5-1微生物馴養1454-5-2生物薄膜反應程序1484-6AOC值在淨水流程及水質分析上之意義153第五章結論與建議1555-1結論1555-2建議157參考文獻參-1圖目錄頁數圖2.1傳統淨水場處理流程圖10圖2.2高級淨水處理流程圖Ⅰ11圖2.3高級淨水處理流程圖Ⅱ11圖2.4高級淨水處理流程圖Ⅲ11圖2.5鹵化乙酸之結構式49圖2.6三鹵甲烷之結構式58圖2.7各物種粒徑大小與各式薄膜孔徑之分佈圖64圖2.8過濾機制示意圖66圖2.9薄膜過濾機制圖68圖2.10側流式與沉浸式薄膜生物反應槽73圖2.11薄膜單元取代之二級生物程序設施項目圖78圖3.1研究流程圖Ⅰ81圖3.2研究流程圖Ⅱ82圖3.3HAAs之實驗分析步驟90圖3.4THMs之實驗分析步驟95圖3.5AOC分析之流程圖100圖3.6P.fluorescensstrainP17104圖3.7Spirillumsp.strainNOX105圖3.8AOC檢量線分析流程圖110圖3.9AOC水樣處理之流程圖112圖3.10生物活性碳薄膜裝置設備圖113圖4.1PseudomonasfluorescencestrainP17於各濃度之μgacetate-C濃度下之生長曲線119圖4.2SpirillumspexiesstrainNOX於各濃度之μgacetate-C濃度下之生長曲線120圖4.3PseudomonasfluorescencestrainP17之最大菌落數μgacetate-C之產率關係121圖4.4SpirillumspexiesstrainNOX之最大菌落數與μgacetate-C之產率關係122圖4.5A流程原水總三鹵甲烷潛勢(THMFP)成份分析圖128圖4.6B流程原水總三鹵甲烷潛勢(THMFP)成份分析圖128圖4.7A流程原水五種鹵化乙酸潛勢(HAA5FP)成份分析圖131圖4.8A流程原水九種鹵化乙酸潛勢(HAA9FP)成份分析圖131圖4.9B流程原水五種鹵化乙酸潛勢(HAA5FP)成份分析圖132圖4.10B流程原水九種鹵化乙酸潛勢(HAA9FP)成份分析圖132圖4.11A流程原水總三鹵甲烷(THMs)成份組成分析圖134圖4.12B流程原水總三鹵甲烷(THMs)成份組成分析圖134圖4.13A流程清水五種鹵化乙酸(HAA5)成份組成分析圖136圖4.14B流程清水五種鹵化乙酸(HAA5)成份組成分析圖136圖4.15A流程清水五種鹵化乙酸(HAA9)成份組成分析圖137圖4.16B流程清水五種鹵化乙酸(HAA9)成份組成分析圖137圖4.17A淨水流程溶解性有機碳(DOC)變化趨勢圖140圖4.18B淨水流程溶解性有機碳(DOC)變化趨勢圖140圖4.19A淨水流程生物可利用有機碳(AOC)變化趨勢圖143圖4.20B淨水流程生物可利用有機碳(AOC)變化趨勢圖143圖4.21A淨水流程AOC-Total、AOC-NOX、AOC-P17比例圖144圖4.22A淨水流程AOC-Total、AOC-NOX、AOC-P17比例圖144圖4.23微生物馴養PAC濃度與DOC相關圖146圖4.24微生物馴養PAC濃度與AOC相關圖146圖4.25連續式生物活性碳薄膜反應HRT與DOC圖152圖4.26連續式生物活性碳薄膜反應HRT與AOC關係152圖4.27HRT與AOC-Total、AOC-NOX、AOC-P17比例153表目錄頁數表2.1NOM組成物種28表2.2P.fluorescensstrainP17及Spirillumsp.strainNOX之特性36表2.3P.fluorescensstrainP17及Spirillumsp.strainNOX菌屬利用基質之差異性比較37表2.3P.fluorescensstrainP17及Spirillumsp.strainNOX菌屬利用基質之差異性比較(續)38表2.3P.fluorescensstrainP17及Spirillumsp.strainNOX菌屬利用基質之差異性比較(續)39表2.4AOC分析方法比較41表2.5AOC-P17及AOC-NOX產率之比較Cellyield(CFU/μgC-Equivalent)42表2.6加氯消毒副產物種類46表2.7鹵化乙酸化合物之物理性質48表2.8各國HAA單一物種之法規值56表2.9三鹵甲烷化合物之物理性質58頁數表2.10國內外飲用水三鹵甲烷之管制值61表2.11薄膜之分類與功能63表2.12各式膜組優缺點比較65表2.13生物薄膜程序與傳統活性污泥法之比較72表3.1水質分析方法彙整84表3.2StrainP17及StrainNOX之鑑定結果108表3.3Chemostatmedium培養液成分114表4.1P.fluorescencestrainP17及Spirillumsp.strainNOX兩株純菌之生化鑑定結果117表4.2P17與NOX對基質利用率之相關研究比較118表4.3高級淨水流程原水水質123表4.4高級淨水流程清水水質124表4.5Chemostatmedium成分145表4.6生物活性碳薄膜反應程序進出流水質特性151 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飲用水水質標準(2004),http://www.epa.gov.tw/j/drinkwater/law/law04.htm.  國圖紙本論文 推文 網路書籤 推薦 評分 引用網址 轉寄                                                                                                                                                                                                                    top 相關論文 相關期刊 熱門點閱論文 1. 混凝吸附對溶解性有機物去除及受預氯影響之研究 2. 以加強混凝去除三鹵甲烷前質 3. 淨水系統對不同分子量消毒副產物前質去除之研究 4. 澄清湖淨水場效能評估與配水管網污染物之分佈及宿命研究 5. 臭氧搭配活性碳處理去除水中有機物之探討 6. 以活性碳生物程序去除水處理系統中生物可利用有機碳及消毒副產物潛勢之研究 7. 探討脫氯對模擬建物自來水配管生物穩定性之影響 8. 利用薄膜生物處理程序去除有機碳 9. 預前臭氧處理及活性碳吸附對自來水加氯消毒副產物之影響   1. 樓基中、蔣本基，(1991)，飲用水中腐植酸氯化反應生成機制之研究，中國環境工程學刊，1(2)，57-64。

2. 樓基中、蔣本基，(1991)，飲用水中腐植酸氯化反應生成機制之研究，中國環境工程學刊，1(2)，57-64。

  1. 以活性碳生物程序去除水處理系統中生物可利用有機碳及消毒副產物潛勢之研究 2. 利用薄膜生物處理程序去除有機碳 3. 利用生物濾床處理飲用水三鹵甲烷、鹵化乙酸與生物可利用有機碳之研究 4. 以淨水程序去除AOC值或吸附去除無機鹽之研究 5. 水中有機物光譜性質在高級淨水處理程序單元之變動 6. 淨水程序與配水管網中生物可分解有機質變化與預測之研究 7. 高級淨水程序消毒副產物之生成研究 8. 應用透地雷達法於地下廢棄埋物檢測之研究 9. 印刷電路板業含銅污泥回收有價金屬之研究 10. 飲用水處理程序中自然有機物之特性及去除之研究 11. 飲用水配水管線中鉛和不鏽鋼之電化腐蝕反應 12. 利用生物濾床去除飲用水中之氨氮、鐵與錳 13. 飲用水配水系統消毒副產物及二氧化鉛溶鉛之健康風險評估 14. 以生物活性碳濾床方法去除水中微量有機物之研究 15. 以類神經網路(AutoNet)模擬淨水場原水有機物濃度及驗證     簡易查詢 | 進階查詢 | 熱門排行 | 我的研究室